It has been a while since I was watching The Prisoner series and reading about it. In that time I also looked up music with Prisoner themes or samples. Here is the result in chronological order:
01 McGoohan’s Blues 1969 by Roy Harper
02 The Prisoner 1980 by The Clash
03 I Helped Patrick McGoohan Escape 1982 by The Times
04 Back In The Village 1984 by Iron Maiden
05 Prisoner 1988 by Iron Maiden
06 The Girl Who Was… Death (epilogue) 1989 by Devil Doll
07 The Prisoner (The Portmeirion Mix) 1989 by Howard Jones
08 We Want Information 1992 by Gravity
09 Speedlearn 1993 by Higher Intelligence Agency
10 #1 1994 by David Shea
11 Information / 32nd Theme Song 1995 by Toenut
12 The Man In The Moon 1996 by Imperial Drag
13 Fall Out 1989 by Mansun
14 Prisoner 2006 by Stanton Warrior
15 Escape From The Village 2007 by Blitzkrieg
16 The Betrayer 2010 by Kai King
17 Shuchu Ryoku Part 3 2010 by Ex.Order
The Spotify version is about the same.